Catalytic Activation of Carbon Dioxide by William M. Ayers

By William M. Ayers

content material: resources and economics of carbon dioxide / Sol J. Barer and Kenneth M. Stern --
Carbon dioxide equilibria / James N. Butler --
Coordination of carbon dioxide to nickel : another theoretical version / R.P. Messmer and H.-J. Freund --
Metal-induced modifications of carbon dioxide / Donald J. Darensbourg, Christopher G. Bauch, and Cesar Ovalles --
Use of stoichiometric reactions within the layout of redox catalyst for carbon dioxide relief / Daniel L. DuBois and Alex Miedaner --
Electrocatalytic carbon dioxide aid / B. Patrick Sullivan, Mitchell R.M. Bruce, Terrence R. O'Toole, C. Mark Bolinger, Elise Megehee, Holden Thorp, and Thomas J. Meyer --
Enzymatic activation of carbon dioxide / Leland C. Allen --
Adsorptive and catalytic homes of carbon monoxide and carbon dioxide over supported steel oxides / D.G. Rethwisch and J.A. Dumesic --
Adsorption and response of carbon dioxide on zirconium dioxide / Ronald G. Silver, Nancy B. Jackson, and John G. Ekerdt --
impression of potassium at the hydrogenation of carbon monoxide and carbon dioxide over supported Rh catalysts / S.D. Worley and C.H. Dai --
Carbon dioxide aid with an electrical box assisted hydrogen insertion response / W.M. Ayers and M. Farley --
Electrochemical relief of aqueous carbon dioxide at electroplated Ru electrodes : investigations towards the mechanism of methane formation / Karl W. Frese, Jr. and David P. Summers --
Electrochemical experiences of carbon dioxide and sodium formate in aqueous ideas / M.H. Miles and A.N. Fletcher --
Electrochemical activation of carbon dioxide / okay. Chandrasekaran and J. O'M. Bockris.

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11. ; Yamamoto, A. : Toyko, Japan, 1982, p 79. 12. Darensbourg, D. J . ; Ovalles, C. Chem. Tech. 1985, 15, 636. 13. Chem. Eng. News, 1985, 63, 10. 14. Czoukowski, M. ; Bayne, A. R. Hydrocarbon Process. 1980, 59, 103. 15. Leonard, J. D. S. Patent 4 299 981 (1981). 16. Ikaraski, T. Chem. Economy & Eng. Rev. 1980, 12, 31 17. Darensbourg, D. ; Rokicki, A. Organometallics 1982, 1, 1685. 18. Slater, S. ; Schumann, B. ; Darensbourg, M. Organometallics 1982, 1, 1662. 19. Darensbourg, D. J . ; Darensbourg, M.

Nobile, C. F. J. Chem. Soc. Dalton Trans. 1977, 708. ; Steinmann, M. Angew. Chem. 1982, 94, 526. Jordan, K. D. J. Phys. Chem. 1984, 88, 2459. Kafafi, Z. ; Hange, R. ; Billups, W. ; Margrave, J. L. J. Am. Chem. Soc. 1983, 105, 3886. ch004 Donald J. Darensbourg, Christopher G. Bauch, and Cesar Ovalles Department of Chemistry, Texas A&M University, College Station, TX 77843 The activation of carbon dioxide by homogeneous and heterogeneous metal catalysts, as well as the nature of the stoichiometric insertion processes of these cata­ lysts, are examined.

5 4. DARENSBOURG ET AL. Metal-Induced 33 Transformations undergone s i g n i f i c a n t advancement, analogous p r o c e s s e s i n v o l v i n g m e t a l - a l k o x i d e s have been l e s s w e l l - i n t e r p r e t e d (32-34). We have r e c e n t l y s y n t h e s i z e d W(C0) 0R~ (R = Ph, C h\CH -m) d e r i v a t i v e s from W(C0) THF and [Et„N][OR] s a l t s (Darensbourg, D. J . ; Sanchez, Κ. ; R h e i n g o l d , A. L. J . Am. Chem. S o c , i n p r e s s ) . I n s o l u t i o n t h e s e s p e c i e s a r e e x t r e m e l y CO l a b i l e , decomposing r e a d i l y t o W„(CO) ( y - 0 R ) ~ i n t h e absence o f a CO atmosphere ( 3 5 ) .

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