Biosynthesis Volume 4 by J D Bu'Lock

By J D Bu'Lock

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Railton and D. 30 Biosynthesis CH20COCH2CH, CO H CH,OH (49) (51) 0-0 (53) R (54)R 155) R CH, CHO = C02H = = and a lactone (56) arising from the epoxide. Hydroxylation of the 2’-ethoxycarbonylethyl ester of ent-kaur-16-en-19-oic acid has been utilizeds6 for an efficient microbiological synthesis of ent-7a-h ydroxykaur- 16-en-19-oic acid. The full paper describing the preparation of fluorogibberellic acid and fluorogibberellin A,, by the microbiological transformation of fluorogibberellin A,, aldehyde with G.

F. Knapp, and T. W. Goodwin, Lipids, 1974, 9, 582. 6 6 W. R. Ness, Lipids, 1974, 9, 596. " J. M. C. Geuns and J. C. Vendrig Phytochemistry, 1974,13,919. 6 8 T. J. Douglas and L. G. , 1974, 54, 238. 70 In fresh slices cycloartenol is heavily labelled, though 24methylenecycloartanol(46) and phytosterols contain no radioactivity. Ageing results HO HO (47) (46) in significant radiolabelling of metabolites of cycloartenol, notably (46) and isofucosterol(47). Free phytosterol content also increases fivefold over the 24 hour period.

J. Patterson, Planta, 1974, 119, 183. P. R. Jefferies, J. R Knox, and T. Ratajczak, Phytochemistry, 1974, 13, 1423. J. Bakker, 1. F. Cook, P. R. Jefferies, and J. R. Knox, Tetrahedron, 1974,30,3631. J. D. Railton and D. 30 Biosynthesis CH20COCH2CH, CO H CH,OH (49) (51) 0-0 (53) R (54)R 155) R CH, CHO = C02H = = and a lactone (56) arising from the epoxide. Hydroxylation of the 2’-ethoxycarbonylethyl ester of ent-kaur-16-en-19-oic acid has been utilizeds6 for an efficient microbiological synthesis of ent-7a-h ydroxykaur- 16-en-19-oic acid.

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